Eur. Phys. J. Appl. Phys.
Volume 57, Number 2, February 2012
|Number of page(s)||8|
|Section||Imaging, Microscopy and Spectroscopy|
|Published online||30 January 2012|
A vibrational dynamics of molecule chain on metallic surface
Laboratoire de Physique et Chimie Quantique, Faculté des Sciences, Université Mouloud Mammeri, BP17 RP, 15000 Tizi-Ouzou, Algeria
2 Laboratoire de Physique de l’État Condensé, Université du Maine, 72085 Le Mans, France
a e-mail: email@example.com
Accepted: 30 November 2011
Published online: 30 January 2012
We investigate the vibration properties of adsorbed nanostructure on the infinite square crystalline surface. The surface is considered as an infinite slab of one atomic layer, and the nanostructure as an isolated diatomic molecule chain on the surface of a cubic lattice which is parallel to y-axis, and takes three different positions: top, hollow and bridge. The vibrational dynamics of the structure is considered within the harmonic approximation framework. The evanescent and propagating vibrational field of the perfect lattice is determined and discussed. The presence of the molecule chain breaks down the translation symmetry in one direction and gives rise to localized states on its neighborhood. The mathematical framework of the matching method is used to analyze the localization phenomena at the nanostructure boundaries. Typical dispersion curves for modes of energies along the inhomogeneity are given with their polarizations. The fine structure of the spectrum and its origins are clearly identifiable, which gives a new insight into the localization problem. Furthermore, the existence and nature of the localized phonons like modes associated with an isolated defect are derived, and the importance of the contribution of these modes to the spectral and states densities is exhibited clearly.
© EDP Sciences, 2012
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